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Comparison of radioactivity data measured in PM10 aerosol samples at two elevated stations in northern Italy during the Fukushima event

TitleComparison of radioactivity data measured in PM10 aerosol samples at two elevated stations in northern Italy during the Fukushima event
Publication TypeArticolo su Rivista peer-reviewed
Year of Publication2012
AuthorsTositti, L., Brattich E., Cinelli Giorgia, Previti A., and Mostacci D.
JournalJournal of Environmental Radioactivity
Volume114
Pagination105-112
ISSN0265931X
KeywordsActivity concentration, Activity levels, adult, aerosol, Aerosol samples, Aerosols, Air Pollutants, air sampling, Airborne particulate, Apennines, article, Artificial radionuclides, Atmospheric activity, Atmospheric movements, atmospheric plume, atmospheric pollution, Atmospheric radioactivity, atmospheric transport, Back-trajectories, beryllium 7, Bologna [Emilia-Romagna], cesium, cesium 134, cesium 137, cesium isotope, comparative study, concentration (composition), concentration (parameters), controlled study, data set, dosimetry, Emilia-Romagna, Fukushima Nuclear Accident, gamma spectrometry, Humans, Infant, iodine, iodine 131, Italy, Japan, lead 210, Local populations, Modena, Natural backgrounds, Natural radionuclides, Northern Apennines, Northern Italy, nuclear accident, Nuclear accidents, particulate matter, plume, Radiation, radiation detection, Radiation Dosage, radiation dose, radiation monitoring, Radioactive, Radioactive plume, radioactive pollution, radioactivity, Radioisotopes, radionuclide, radium 226, Spatial patterns, tsunami, vertical mixing
Abstract

The follow-up of Fukushima radioactive plume resulting from the 11th March 2011 devastating tsunami is discussed for two Italian stations in the northern Apennines: Mt. Cimone (Modena) and Montecuccolino (Bologna). Radioactivity data collected at both stations are described, including comparison between local natural background of airborne particulate and artificial radioactivity referable to the arrival of the radioactive plume and its persistence and evolution. Analysis of back-trajectories was used to confirm the arrival of artificial radionuclides following atmospheric transport and processing. The Fukushima plume was first detected on 3rd April 2011 when high volume sampling revealed the presence of the artificial radionuclides 131I, 137Cs and 134Cs. The highest activity concentrations of these nuclides were detected on 5th April 2011 at the Montecuccolino site. Fukushima radioactivity data at the two stations were usually comparable, suggesting a good vertical mixing of the plume; discrepancies were occasional and attributed to different occurrence of wet removal, typically characterized by a scattered spatial pattern. To understand the relevance to the local population of the extra dose due to the Fukushima plume, atmospheric activities of the related artificial nuclides were compared to those of the main natural radionuclides in ambient particulate, and found to be lower by over one order of magnitude. Radiation doses referable to Fukushima, maximized for a whole year occurrence at the highest activity level observed at our stations in the weeks affected by the Japanese plume, were estimated at 1.1 μSv/year. © 2012 Elsevier Ltd.

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URLhttps://www.scopus.com/inward/record.uri?eid=2-s2.0-84866618826&doi=10.1016%2fj.jenvrad.2012.01.016&partnerID=40&md5=d67880e0ef87a91226602533073c34da
DOI10.1016/j.jenvrad.2012.01.016
Citation KeyTositti2012105