A climatology of 7Be in surface air in European Union

TitleA climatology of 7Be in surface air in European Union
Publication TypeArticolo su Rivista peer-reviewed
Year of Publication2015
AuthorsHernández-Ceballos, M.Á., Cinelli Giorgia, M. Ferrer Marín, Tollefsen T., De Felice L., Nweke E., Tognoli P.V., Vanzo S., and de Cort M.
JournalJournal of Environmental Radioactivity
Volume141
Pagination62-70
ISSN0265931X
KeywordsActivity concentration, air, air pollutant, Air Pollutants, Air pollution, air sampling, altitude, analysis, article, Atmospheric boundary layer, atmospheric deposition, Atmospheric radioactivity, Beryllium, beryllium 7, beryllium isotope, boundary layer, climate, Climate change, concentration (composition), concentration (parameters), cosmogenic radionuclide, data base, database, Environmental monitoring, Europe, European Union, Isotopes, latitude, Maximum concentrations, nuclear accident, radiation monitoring, Radioactive, radioisotope, Radioisotopes, season, seasonal variation, Seasons, Solar activity, solar cycle, Solar energy, Spatial and temporal distribution, spatial distribution, spatiotemporal analysis, summer, Temporal and spatial distribution, variance analysis, vertical distribution, Vertical distributions, winter
Abstract

This study presents a European-wide analysis of the spatial and temporal distribution of the cosmogenic isotope 7Be in surface air. This is the first time that a long term database of 34 sampling sites that regularly provide data to the Radioactivity Environmental Monitoring (REM) network, managed by the Joint Research Centre (JRC) in Ispra, is used. While temporal coverage varies between stations, some of them have delivered data more or less continuously from 1984 to 2011. The station locations were considerably heterogeneous, both in terms of latitude and altitude, a range which should ensure a high degree of representativeness of the results. The mean values of 7Be activity concentration presented a spatial distribution value ranging from 2.0 to 5.4mBq/m3 over the European Union. The results of the ANOVA analysis of all 7Be data available indicated that its temporal and spatial distributions were mainly explained by the location and characteristic of the sampling sites rather than its temporal distribution (yearly, seasonal and monthly). Higher 7Be concentrations were registered at the middle, compared to high-latitude, regions. However, there was no correlation with altitude, since all stations are sited within the atmospheric boundary layer. In addition, the total and yearly analyses of the data indicated a dynamic range of 7Be activity for each solar cycle and phase (maximum or minimum), different impact on stations having been observed according to their location. Finally, the results indicated a significant seasonal and monthly variation for 7Be activity concentration across the European Union, with maximum concentrations occurring in the summer and minimum in the winter, although with differences in the values reached. The knowledge of the horizontal and vertical distribution of this natural radionuclide in the atmosphere is a key parameter for modelling studies of atmospheric processes, which are important phenomena to be taken into account in the case of a nuclear accident. © 2014 The Authors.

Notes

cited By 42

URLhttps://www.scopus.com/inward/record.uri?eid=2-s2.0-84919935883&doi=10.1016%2fj.jenvrad.2014.12.003&partnerID=40&md5=87db50c7f68fef91155f0273337a692f
DOI10.1016/j.jenvrad.2014.12.003